Carbonyl Sulphide (OCS) Variability with Latitude in the Atmosphere     

Gisèle Krysztofiak  Yao Veng Té  Gwenaël Berthet  Geoffrey C. Toon  Fabrice Jégou 《大气与海洋》2015,53(1):89-101

Abstract

Carbonyl sulphide (OCS) is an important precursor of sulphate aerosols and consequently a key species in stratospheric ozone depletion. The SPectromètre InfraRouge d'Absorption à Lasers Embarqués (SPIRALE) and shortwave infrared (SWIR) balloon-borne instruments have flown in the tropics and in the polar Arctic, and ground-based measurements have been performed by the Qualité de l'Air (QualAir) Fourier Transform Spectrometer in Paris. Partial and total columns and vertical profiles have been obtained to study OCS variability with altitude, latitude, and season. The annual total column variation in Paris reveals a seasonal variation with a maximum in April–June and a minimum in November–January. Total column measurements above Paris and from SWIR balloon-borne instrument are compared with several MkIV measurements, several Network for the Detection of Atmospheric Composition Change (NDACC) stations, aircraft, ship, and balloon measurements to highlight the OCS total column decrease from tropical to polar latitudes. OCS high-resolution in situ vertical profiles have been measured for the first time in the altitude range between 14 and 30?km at tropical and polar latitudes. OCS profiles are compared with Atmospheric Chemistry Experiment (ACE) satellite measurements and show good agreement. Using the correlation between OCS and N₂O from SPIRALE, the OCS stratospheric lifetime has been accurately determined. We find a stratospheric lifetime of 68?±?20 years at polar latitudes and 58?±?14 years at tropical latitudes leading to a global stratospheric sink of 49?±?14?Gg?S?y^?1.  相似文献   

Atmospheric Circulation Changes in Response to an Observed Stratospheric Zonal Ozone Anomaly     

Dieter H. W. Peters  Andrea Schneidereit  Marianne Bügelmayer  Christoph Zülicke  Ingo Kirchner 《大气与海洋》2015,53(1):74-88

Abstract

In a sensitivity study, the influence of an observed stratospheric zonal ozone anomaly on the atmospheric circulation was investigated using the Fifth Generation European Centre Hamburg Model (ECHAM5) which is a general circulation model. The model was run from 1960 to 1999 (40 years) with a mean seasonal cycle of zonally symmetric ozone. In order to isolate the induced dynamical influence of the observed zonally asymmetric part of the three-dimensional stratospheric ozone, a second run was performed for the boreal extratropics using prescribed monthly means from the 40-year reanalysis dataset from the European Centre for Medium-range Weather Forecasts (ERA-40). The main findings are the interdecadal westward shift of the polar vortex at about 65°N and a significant increase in the number of stratospheric sudden warmings during the 1980–99 period. Under the action of zonally asymmetric ozone a decrease in the Arctic Oscillation was identified between the mid-1980s and the mid-1990s. The lag correlation between the mean Arctic Oscillation at the surface and the daily stratospheric northern annular mode increased in mid-winter. Furthermore, we examined the influence of the stratospheric zonal ozone anomaly on Rossby wave breaking in the upper troposphere and found a significant westward shift of poleward Rossby wave breaking events over western Europe in the winter. By this we show that the stratospheric zonal ozone anomaly has a strong influence on the tropospheric circulation as a result of enhanced dynamical coupling processes.  相似文献   

Characterizing the effects of policy instruments on the future costs of carbon capture for coal power plants     

Gregory F. Nemet  Erin Baker  Bob Barron  Samuel Harms 《Climatic change》2015,133(2):155-168

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Hot deontology and cold consequentialism – an empirical exploration of ethical reasoning among climate change negotiators     

Manjana?MilkoreitEmail author 《Climatic change》2015,133(3):397-406

Philosophers, political theorists and cognitive scientists have applied the traditional distinction between deontology and consequentialism to determine ethical responsibilities – usually of states – to take action in response to climate change. Most of this work is either purely conceptual or based on experiments with individuals, who are not part of the global political process. This paper makes two contributions to this debate. First, based on interview data I describe existing patterns of ethical reasoning among global political actors rather than groups selected for lab experiments. Integrating theories of risk perceptions, international relations and moral philosophy, I identify both deontological and consequentialist cognitive patterns, and examine their constitutive elements. My second contribution concerns the role of emotion in moral reasoning. Using the same qualitative data, I offer support for a controversial argument about the emotional nature of deontological reasoning. Further, I argue that many negotiators experience climate change not as an impersonal threat posed by the environment, but rather as an “up, close and personal” threat, over which other negotiation participants have significant control.  相似文献   

Border Tax adjustment – legal perspective     

Rolf H. Weber 《Climatic change》2015,133(3):407-417

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Climate change,climate justice and the application of probabilistic event attribution to summer heat extremes in the California Central Valley     

Roberto Mera  Neil Massey  David E. Rupp  Philip Mote  Myles Allen  Peter C. Frumhoff 《Climatic change》2015,133(3):427-438

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Climate change impacts on streamflow availability for the Athabasca Oil Sands     

Doris N. S. Leong  Simon D. Donner 《Climatic change》2015,133(4):651-663

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Vulnerability assessment for loss of access to drinking water due to extreme weather events   总被引：1，自引：0，他引：1  

Jeanne Luh  Elizabeth C. Christenson  Aizhan Toregozhina  David A. Holcomb  Tucker Witsil  Laura R. Hamrick  Edema Ojomo  Jamie Bartram 《Climatic change》2015,133(4):665-679

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A multi-proxy reconstruction of spatial and temporal variations in Asian summer temperatures over the last millennium   总被引：1，自引：0，他引：1  

Feng?Shi  Quansheng?GeEmail author  Bao?Yang  Jianping?Li  Fengmei?Yang  Fredrik?Charpentier?Ljungqvist  Olga?Solomina  Takeshi?Nakatsuka  Ninglian?Wang  Sen?Zhao  Chenxi?Xu  Keyan?Fang  Masaki?Sano  Guoqiang?Chu  Zexin?Fan  Narayan?P.?Gaire  Muhammad?Usama?Zafar 《Climatic change》2015,131(4):663-676

To investigate climate variability in Asia during the last millennium, the spatial and temporal evolution of summer (June–July–August; JJA) temperature in eastern and south-central Asia is reconstructed using multi-proxy records and the regularized expectation maximization (RegEM) algorithm with truncated total least squares (TTLS), under a point-by-point regression (PPR) framework. The temperature index reconstructions show that the late 20th century was the warmest period in Asia over the past millennium. The temperature field reconstructions illustrate that temperatures in central, eastern, and southern China during the 11th and 13th centuries, and in western Asia during the 12th century, were significantly higher than those in other regions, and comparable to levels in the 20th century. Except for the most recent warming, all identified warm events showed distinct regional expressions and none were uniform over the entire reconstruction area. The main finding of the study is that spatial temperature patterns have, on centennial time-scales, varied greatly over the last millennium. Moreover, seven climate model simulations, from the Coupled Model Intercomparison Project Phase 5 (CMIP5), over the same region of Asia, are all consistent with the temperature index reconstruction at the 99 % confidence level. Only spatial temperature patterns extracted as the first empirical orthogonal function (EOF) from the GISS-E2-R and MPI-ESM-P model simulations are significant and consistent with the temperature field reconstruction over the past millennium in Asia at the 90 % confidence level. This indicates that both the reconstruction and the simulations depict the temporal climate variability well over the past millennium. However, the spatial simulation or reconstruction capability of climate variability over the past millennium could be still limited. For reconstruction, some grid points do not pass validation tests and reveal the need for more proxies with high temporal resolution, accurate dating, and sensitive temperature signals, especially in central Asia and before AD 1400.  相似文献   

Increasing Northern Hemisphere water deficit     

Gregory J. McCabe  David M. Wolock 《Climatic change》2015,132(2):237-249

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